Results/Conclusions Comparisons of C dynamics in harvested ecosystems that include temperate timberlands and croplands revealed general differences in C sequestration among ecosystem types. The annual C sequestration rate of perennial grass crops is greater than that of other harvested ecosystems, but the efficiency of C assimilation is dependent on management choices in all cases. The timing of harvest significantly affects the stability of C storage in most ecosystems. The relative potential for C sequestration in harvested ecosystems is directly relevant to new policies governing greenhouse gas reduction and biomass for bioenergy.